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RAS Chemistry & Material ScienceЖурнал неорганической химии Russian Journal of Inorganic Chemistry

  • ISSN (Print) 0044-457X
  • ISSN (Online) 3034-560X

Sorption of Radionuclides on Amorphous and Crystalline Cerium(IV) Phosphates

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PII
10.31857/S0044457X23601207-1
DOI
10.31857/S0044457X23601207
Publication type
Status
Published
Authors
T. O. Kozlova
  • Affiliation: Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences
Volume/ Edition
Volume 68 / Issue number 11
Pages
1515-1522
Abstract
The sorption properties of amorphous cerium(IV) hydrogen phosphate and crystalline phases NH4Ce2(PO4)3, (NH4)2Ce(PO4)2·H2O, and Ce(OH)PO4 towards the 243Am(III), 232Th(IV), 237Np(V), and 233, 238U(VI) radionuclides were studied in aqueous media at pH 1, 4, 7, and 10 for 24 h. The highest degree of sorption (up to 100%) was found for amorphous cerium(IV) hydrogen phosphate. The pH dependences of radionuclide sorption for crystalline compounds were shown to be similar to one another: the highest sorption was observed at pH 7 (up to 100% for 243Am(III)), while the lowest values were observed for pH 10 and 1. An exception was provided by 237Np(V), the sorption of which was close to zero in the pH range of 1–7 and reached 60% at pH 10. Keeping amorphous and crystalline cerium(IV) phosphates in acid medium leads to quantitative desorption of all of the tested radionuclides within the first 5 h.
Keywords
жидкие радиоактивные отходы сорбенты адсорбция фосфаты РЗЭ
Date of publication
01.11.2023
Year of publication
2023
Number of purchasers
0
Views
41

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