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RAS Chemistry & Material ScienceЖурнал неорганической химии Russian Journal of Inorganic Chemistry

  • ISSN (Print) 0044-457X
  • ISSN (Online) 3034-560X

Chemical Generation And Reactivity Of Highly Oxidized Oxo-Species Of Water-Soluble µ-Carbide Dimer Ruthenium(IV)Phthalocyaninate

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PII
10.31857/S0044457X24060058-1
DOI
10.31857/S0044457X24060058
Publication type
Article
Status
Published
Authors
S. V. Zaitseva
  • Affiliation:
    G. A. Krestov Institute of Solution Chemistry of the Russian Academy of Science
    N.D. Zelinsky Institute of Organic Chemistry Russian Academy of Sciences
Volume/ Edition
Volume 69 / Issue number 6
Pages
829-843
Abstract
The chemical generation of highly oxidized species of µ-carbido dimer water-soluble ruthenium sulfophthalocyaninate in reaction with tert-butyl hydroperoxide was studied using spectral methods. The regularities of the active species formation have been established and a reaction mechanism has been proposed. The coordinating ability of the dimeric complex is shown to determine the possibility of the π-radical cation and diradical cation species formation. The influence of peroxide concentration and pH of the medium on the type of the generated active species capable of oxidizing not only synthetic dye, but also organic peroxide, is demonstrated.
Keywords
фталоцианин рутений биядерный комплекс оксоформа катион-радикал
Date of publication
15.06.2024
Year of publication
2024
Number of purchasers
0
Views
47

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